This dataset contains geochemical data for unconsolidated sediments (stream sediments, lake sediments, etc.) collected by U.S. Geological Survey (USGS) personnel and analyzed in the analytical laboratories of the Geologic Division of the USGS. These data represent analyses of sediment samples collected in support of various USGS programs. The data were originally entered into the in-house Rock Analysis Storage System (RASS) database which was used by the Geologic Division from the early-1970's through the late-1980's to archive geochemical data. An unpublished CD-ROM was developed in 1996 that contains the RASS data in GSSEARCH format. That CD was used to generate this data set.